<p>Title : </p>
<p>Rational Design of Functional Materials: A Chemist's Approach</p>
<p>Abstract :</p>
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<p> </p>
<p class="MsoNormal" style="text-align: justify;"><span style="color: black;">Functional materials have assumed prominent position in several high tech areas. Such materials are not classified on the basis of their origin, nature of bonding or processing techniques but are classified on the basis of functions which they can perform.<span style="mso-spacerun: yes;">  </span></span>The synthesis of such materials has been a challenge and also opportunity to chemists. New functional materials can be designed by interplay of synthesis and crystallographic structure. Other approaches for design of these materials are defects engineering and concepts of hybrids. Unconventional synthetic routes play an important role in this direction as many of these new materials are metastable and hence it is not possible to prepare them by conventional solid state synthesis.<span style="mso-spacerun: yes;">  </span>We have prepared [1-18] a number of new functional materials guided by crystallographic approach coupled with novel synthesis protocols. Some typical materials which will be discussed in this talk are La<sub>1-x</sub>Ce<sub>x</sub>CrO<sub>3</sub> (materials with tunable band gap and magnetic properties), CeScO<sub>3</sub> (with unusual reversible conversion to fluorite lattice), Gd<sub>1-x</sub>Y<sub>x</sub>InO<sub>3</sub>, GdSc<sub>1-x</sub>In<sub>x</sub>O<sub>3</sub>, <span style="mso-bidi-font-weight: bold;">YIn<sub>1-x</sub>Fe<sub>x</sub>O<sub>3</sub> </span>(tunable dielectrics) and several lead free relaxor materials. Perovskite and fluorite-type materials with trivalent Ce<sup>3+</sup> were successfully prepared from suitable precursor powders by a controlled heating under low p<sub>O2.</sub> Several interesting pyrochlore based oxygen storage materials, viz. Ce<sub>2</sub>Zr<sub>2</sub>O<sub>7+x</sub> (x = 0.0 to 1.0), Gd<sub>2-x</sub>Ce<sub>x</sub>Zr<sub>2</sub>O<sub>7 </sub>andGd<sub>2-x</sub>Ce<sub>x</sub>Zr<sub>2-x</sub>Al<sub>x</sub>O<sub>7</sub> (x = 0.0 to 2.0) have been prepared, which have shown interesting redox catalysis. The simple concepts like r<sub>A</sub>/r<sub>B</sub> ratio of A<sub>2</sub>B<sub>2</sub>O<sub>7</sub> pyrochlores could be used to tailor the functional properties. The major focus of this talk will be on the role of synthesis, novel properties exhibited by these functional materials, and their crystallographic correlation.</p>
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<p class="MsoNormal"><strong><span style="font-size: 11.0pt;">Our recent publications in the field functional materials</span></strong></p>
<p> </p>
<p><span style="font-size: 11.0pt; mso-bidi-font-family: Arial;">[1]<span style="mso-no-proof: yes;"> <span style="mso-spacerun: yes;"> </span>Chem. Mater. 21 (2009) 125</span></span></p>
<p><span style="font-size: 11.0pt; mso-bidi-font-family: Arial;">[2] <span style="mso-spacerun: yes;"> </span></span><span style="font-size: 11.0pt; mso-bidi-font-family: Arial; mso-ansi-language: DE;" lang="DE">J</span><span style="font-size: 11.0pt; mso-ansi-language: DE;" lang="DE">. Phys. Chem. C 113 (2009) 12663</span></p>
<p class="MsoNormal"><span style="font-size: 11.0pt; mso-ansi-language: SV;" lang="SV">[3] <span style="mso-spacerun: yes;"> </span>Inorg. </span><span style="font-size: 11.0pt; mso-ansi-language: DE;" lang="DE">Chem. 48 (2009) 11691</span></p>
<p> </p>
<p class="MsoNormal"><span style="font-size: 11.0pt; mso-ansi-language: DE;" lang="DE">[4]<span style="mso-spacerun: yes;">  </span>Inorg. </span><span style="font-size: 11.0pt;">Chem. 49 (2010) 10415</span></p>
<p> </p>
<p class="MsoNormal"><span style="font-size: 11.0pt;">[5]<span style="mso-spacerun: yes;">  </span>Inorg. Chem 49 (2010) 1152 </span></p>
<p> </p>
<p><span style="font-size: 11.0pt;">[6] <span style="mso-spacerun: yes;"> </span>Chem.- A Eur. J.17 (2011) 12310</span></p>
<p> </p>
<p class="MsoNormal"><span style="font-size: 11.0pt; mso-fareast-font-family: 'MS Mincho'; mso-bidi-font-family: TT10C25o00; mso-fareast-language: JA; mso-bidi-language: BN;">[7] <span style="mso-spacerun: yes;"> </span>Chem. Mater. </span><em><span style="font-size: 11.0pt; color: black; font-style: normal;">24</span></em><span style="font-size: 11.0pt;"> (2012)<span style="color: black;"> 2186</span></span></p>
<p> </p>
<p class="MsoNormal"><span style="font-size: 11.0pt; mso-ansi-language: SV;" lang="SV">[8]<span style="mso-spacerun: yes;">  </span>Analysts 137 (2012) 760 </span></p>
<p> </p>
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<p class="MsoNormal" style="margin-left: 30.0pt; text-indent: -30.0pt; tab-stops: 30.0pt 60.0pt 1.25in 120.0pt 150.0pt 2.5in 210.0pt 240.0pt 3.75in 300.0pt 330.0pt 5.0in 390.0pt 420.0pt 6.25in 480.0pt 510.0pt 7.5in 570.0pt 600.0pt 8.75in 660.0pt 690.0pt 10.0in 750.0pt 780.0pt 11.25in 840.0pt 870.0pt 12.5in;"><span style="font-size: 11.0pt;">[11]<span style="mso-spacerun: yes;">  </span>J. Phys. Chem. C<span style="mso-spacerun: yes;">  </span>117 (2013) 2382</span></p>
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