<p><strong><span style="text-decoration: underline;">Title</span> :</strong> </p>
<h3>Adaptive Pores: Reversible Pore Engineering of Mesoporous Silica</h3>
<p><strong><span style="text-decoration: underline;">Abstract</span> :</strong></p>
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<p class="MsoNormal" style="line-height: normal; text-align: justify;"><span style="font-size: 12.0pt;" lang="EN-IN">Non-covalent and dynamic covalent methods were used to reversibly modify the pore size and philicity of mesoporous silica. In the non-covalent approach, the strong, charge-transfer interactions between pyranine and viologen moieties were usedfor reversible pore engineering.The fast binding of donors enabled quick and facile functionalization at room temperature. </span><span style="font-size: 12.0pt; mso-ansi-language: EN-US; mso-bidi-font-style: italic;">The viologen based charge transfer modules were employed in electrostatic gating of ion transport through the nanochannels (&lt;10 nm)<span style="mso-spacerun: yes;">  </span>in mesoporous silica. The polarity of ion transport was switched from anion selective to cation selective through ambipolar stage by controlling the extent of pyranine bound to the viologen. Further, the ion transport could be regulated with respect to pH by selecting a donor (coronenetetracarboxylate) with pH responsive functional groups. </span><span style="font-size: 12.0pt; mso-ansi-language: EN-US;">In the dynamic covalent approach, the reversible bonding between amine and aldehyde has been utilized to reverse the pore properties of silica. </span><span style="font-size: 12.0pt;" lang="EN-IN">The modularity of the approach enables modification of nanopores with custom designed compositions, components and functions.</span></p>
<p class="MsoNormal" style="line-height: normal; text-align: justify;" align="left"><span style="font-size: 12.0pt; mso-fareast-font-family: Calibri; mso-fareast-theme-font: minor-latin; mso-ansi-language: EN-US;">References:</span></p>
<p class="MsoNormal" style="line-height: normal; text-align: justify;" align="left"><span style="font-size: 12.0pt; mso-fareast-font-family: Calibri; mso-fareast-theme-font: minor-latin; mso-ansi-language: EN-US;">1.<span style="mso-spacerun: yes;">  </span>B. V. V. S. Pavan Kumar, K. V. Rao, T. Soumya, S. J. George</span></p>
<p class="MsoNormal" style="line-height: normal; text-align: justify;" align="left"><span style="font-size: 12.0pt; mso-fareast-font-family: Calibri; mso-fareast-theme-font: minor-latin; mso-ansi-language: EN-US;">    and M. Eswaramoorthy, ,<span style="mso-bidi-font-weight: bold;">J. Am. Chem. Soc., </span> 135, 10902 -</span></p>
<p class="MsoNormal" style="line-height: normal; text-align: justify;" align="left"><span style="font-size: 12.0pt; mso-fareast-font-family: Calibri; mso-fareast-theme-font: minor-latin; mso-ansi-language: EN-US;">    10905 (2013)</span></p>
<p class="MsoNormal" style="line-height: normal; text-align: justify;"><span style="font-size: 12.0pt;" lang="EN-IN">2. B. V. V. S. Pavan Kumar, K. Venkata Rao, S. Sampath, </span></p>
<p class="MsoNormal" style="line-height: normal; text-align: justify;"><span style="font-size: 12.0pt;" lang="EN-IN">   S. J. George and M. Eswaramoorthy,<span style="mso-spacerun: yes;">  </span>Angew. Chem. Int. Ed.,</span></p>
<p class="MsoNormal" style="line-height: normal; text-align: justify;"><span style="font-size: 12.0pt;" lang="EN-IN">   53, 13073-13077<span style="mso-spacerun: yes;">  </span>(2014).<span style="mso-spacerun: yes;">  </span></span></p>