<h3>Title</h3>
<h3><span style="font-size: 12.16px;">Design Strategies Towards Stabilization of Organic Radical Ions and their Electroactive Partners</span></h3>
<p><strong><span style="font-size: 12.16px;"><span style="text-decoration: underline;">Abstract</span> :</span></strong></p>
<p class="MsoNormal" style="text-align: justify;"><span style="font-family: Symbol; mso-ascii-font-family: 'Times New Roman'; mso-fareast-font-family: Meiryo; mso-hansi-font-family: 'Times New Roman'; mso-char-type: symbol; mso-symbol-font-family: Symbol;" lang="EN-US"><span style="mso-char-type: symbol; mso-symbol-font-family: Symbol;">p</span></span><span style="mso-fareast-font-family: Meiryo;" lang="EN-US">-conjugated molecules are intriguing building blocks to realize diverse range of closed and open-shell molecular materials.<sup>1</sup> The major challenge facing their applications is the intrinsic reactivity of highly electron-deficient and electron-rich molecules in the neutral and radical ion forms. In this context, the naphthalenediimide (NDI) and the perylenediimide (PDI) </span><span style="font-family: Symbol; mso-ascii-font-family: 'Times New Roman'; mso-fareast-font-family: Meiryo; mso-hansi-font-family: 'Times New Roman'; mso-char-type: symbol; mso-symbol-font-family: Symbol;" lang="EN-US"><span style="mso-char-type: symbol; mso-symbol-font-family: Symbol;">p</span></span><span style="mso-fareast-font-family: Meiryo;" lang="EN-US">-scaffolds provide an intriguing platform to design new electro-active molecules.<sup>2</sup></span></p>
<p class="MsoNormal" style="text-align: justify;"><span style="text-indent: 36pt;"> </span></p>
<p class="MsoNormal" style="text-align: justify;"><span style="text-indent: 36pt;">In this talk, we would discuss how the arylenediimide scaffolds integrated with specific design elements</span><sup style="text-indent: 36pt;">3a</sup><span style="text-indent: 36pt;"> can be utilized to synthesize and isolate new ambient stable radical ions. We have recently extended our efforts in synthetic spin chemistry towards the development of eco-friendly synthetic protocols towards radical ions.</span><sup style="text-indent: 36pt;">3b</sup><span style="text-indent: 36pt;"> Along with this, we recently isolated new </span><em style="text-indent: 36pt;">planar</em><span style="text-indent: 36pt;"> as well as </span><em style="text-indent: 36pt;">twisted</em><span style="text-indent: 36pt;"> ambient stable radical anions as well as the strongest electron acceptors with calculated LUMO of -5.2 eV.</span><sup style="text-indent: 36pt;">4a,b </sup><span style="text-indent: 36pt;">Considering the other end of the electrochemical window, we have been able to isolate highly electron-rich, di-reduced NDI systems, which have an unusual doubly zwitterionic molecular structure and redox switchable aromatic-antiaromatic sites.</span><sup style="text-indent: 36pt;">5</sup><span style="text-indent: 36pt;"> In short, we would discuss the possibilities to expand the electrochemical window of the arylenediimides maintaining their ambient stability. We believe their excited states would be of interest for photocatalysis and other relevant opto-electronic applications.</span></p>
<p class="MsoNormalCxSpLast" style="margin-right: -3.1pt; mso-add-space: auto; text-align: justify; text-indent: 36.0pt;"><span style="mso-fareast-font-family: Meiryo;" lang="EN-US"> </span></p>
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<p class="E4References" style="margin-left: 18.0pt; text-indent: -18.0pt; line-height: normal; mso-list: l0 level1 lfo1; tab-stops: 12.0pt;"><!--[if !supportLists]--><span style="font-size: 10.0pt; mso-fareast-font-family: 'Times New Roman'; mso-ansi-language: EN-US; mso-fareast-language: ZH-CN;" lang="EN-US"><span style="mso-list: Ignore;">1.<span style="font: 7.0pt 'Times New Roman';">   </span></span></span><!--[endif]--><span style="font-size: 10.0pt;" lang="EN-GB">Morita, </span><span style="font-size: 10.0pt; mso-ansi-language: EN-US;" lang="EN-US">Y.; </span><span style="font-size: 10.0pt;" lang="EN-GB">Suzuki,</span><span style="font-size: 10.0pt; mso-ansi-language: EN-US;" lang="EN-US"> S.;</span><span style="font-size: 10.0pt;" lang="EN-GB"> Sato,</span><span style="font-size: 10.0pt; mso-ansi-language: EN-US;" lang="EN-US"> K.;</span><span style="font-size: 10.0pt;" lang="EN-GB"> Takui,</span><span style="font-size: 10.0pt; mso-ansi-language: EN-US;" lang="EN-US"> T.</span><em style="mso-bidi-font-style: normal;"><span style="font-size: 10.0pt;" lang="EN-GB">Nature Chem</span></em><span style="font-size: 10.0pt;" lang="EN-GB">. <strong style="mso-bidi-font-weight: normal;">2011</strong>, <em style="mso-bidi-font-style: normal;">3</em>, 197</span><span style="font-size: 10.0pt; mso-fareast-font-family: Calibri; color: #232021; mso-ansi-language: EN-IN; mso-fareast-language: EN-US; mso-bidi-font-weight: bold;">.</span></p>
<p class="E4References" style="margin-left: 18.0pt; text-indent: -18.0pt; line-height: normal; mso-list: l0 level1 lfo1; tab-stops: 12.0pt;"><!--[if !supportLists]--><span class="listitem-data4"><span style="font-size: 10.0pt; mso-fareast-font-family: 'Times New Roman'; mso-ansi-language: EN-US; mso-fareast-language: ZH-CN;" lang="EN-US"><span style="mso-list: Ignore;">2.<span style="font: 7.0pt 'Times New Roman';">   </span></span></span></span><!--[endif]--><em><span style="font-size: 10.0pt; mso-fareast-font-family: Calibri; color: #232021; mso-ansi-language: EN-IN; mso-fareast-language: EN-US; mso-bidi-font-weight: bold;">A review on electron-poor arylenediimides</span></em><span style="font-size: 10.0pt; mso-fareast-font-family: Calibri; color: #232021; mso-ansi-language: EN-IN; mso-fareast-language: EN-US; mso-bidi-font-weight: bold;">: Kumar, S.; Shukla, J.; Kumar, Y.; Mukhopadhyay, P. </span><strong><em><span style="font-size: 10.0pt; mso-ansi-language: EN; font-weight: normal; mso-bidi-font-weight: bold;" lang="EN">Org. Chem. Front.</span></em></strong><span class="listitem-data4"><span style="font-size: 10.0pt; mso-ansi-language: EN;" lang="EN">, <strong style="mso-bidi-font-weight: normal;">2018</strong>, <em style="mso-bidi-font-style: normal;">5</em>, 2254.</span></span></p>
<p class="E4References" style="margin-left: 18.0pt; text-indent: -18.0pt; line-height: normal; mso-list: l0 level1 lfo1; tab-stops: 12.0pt;"><!--[if !supportLists]--><span style="font-size: 10.0pt; mso-fareast-font-family: 'Times New Roman'; mso-ansi-language: EN-US; mso-fareast-language: ZH-CN;" lang="EN-US"><span style="mso-list: Ignore;">3.<span style="font: 7.0pt 'Times New Roman';">   </span></span></span><!--[endif]--><span style="font-size: 10.0pt; mso-fareast-font-family: Calibri; color: #232021; mso-ansi-language: EN-IN; mso-fareast-language: EN-US; mso-bidi-font-weight: bold;">a) Kumar, S.; Ajayakumar, M. R.; Hundal, G.; Mukhopadhyay, P. <em style="mso-bidi-font-style: normal;">J. Am. Chem. Soc</em>. <strong>2014</strong>, <em style="mso-bidi-font-style: normal;">136</em>, 12004; b) Kumar, S.; Mukhopadhyay, P. <em style="mso-bidi-font-style: normal;">Green</em>. <em style="mso-bidi-font-style: normal;">Chem</em>. <strong>2018</strong>, <em style="mso-bidi-font-style: normal;">20</em>, 4620.</span></p>
<p class="E4References" style="margin-left: 18.0pt; text-indent: -18.0pt; line-height: normal; mso-list: l0 level1 lfo1; tab-stops: 12.0pt;"><!--[if !supportLists]--><span style="font-size: 10.0pt; mso-fareast-font-family: 'Times New Roman'; mso-ansi-language: EN-US; mso-fareast-language: ZH-CN;" lang="EN-US"><span style="mso-list: Ignore;">4.<span style="font: 7.0pt 'Times New Roman';">   </span></span></span><!--[endif]--><span style="font-size: 10.0pt; mso-fareast-font-family: Calibri; color: #232021; mso-ansi-language: EN-IN; mso-fareast-language: EN-US; mso-bidi-font-weight: bold;">a) Kumar, Y.; Kumar, S.; Mandal, K.; Mukhopadhyay, P<em style="mso-bidi-font-style: normal;">. Angew. Chem. Int. Ed</em>. <strong>2018</strong>, <em style="mso-bidi-font-style: normal;">57</em>, 16318; b) </span><span style="font-size: 10.0pt; color: black;" lang="EN-GB">Kumar, </span><span style="font-size: 10.0pt; color: black; mso-ansi-language: EN-US;" lang="EN-US">Y.; </span><span style="font-size: 10.0pt; color: black;" lang="EN-GB">Kumar,</span><span style="font-size: 10.0pt; color: black; mso-ansi-language: EN-US;" lang="EN-US"> S.;</span><span style="font-size: 10.0pt; color: black;" lang="EN-GB">Bansal, D.</span><span style="font-size: 10.0pt; color: black; mso-ansi-language: EN-US;" lang="EN-US">;</span><span style="font-size: 10.0pt; color: black;" lang="EN-GB"> Mukhopadhyay, P. <em style="mso-bidi-font-style: normal;">Org. Lett.</em> </span><strong style="mso-bidi-font-weight: normal;"><span style="font-size: 10.0pt; color: black; mso-ansi-language: EN-US;" lang="EN-US">2019</span></strong><span style="font-size: 10.0pt; color: black; mso-ansi-language: EN-US;" lang="EN-US">,</span><em style="mso-bidi-font-style: normal;"><span style="font-size: 10.0pt; color: black;" lang="EN-GB">21</span></em><span style="font-size: 10.0pt; color: black; mso-ansi-language: EN-US;" lang="EN-US">,</span><span style="font-size: 10.0pt; color: black;" lang="EN-GB">2185.</span></p>
<p class="E4References" style="margin-left: 18.0pt; text-indent: -18.0pt; line-height: normal; mso-list: l0 level1 lfo1; tab-stops: 12.0pt;"><!--[if !supportLists]--><span style="font-size: 10.0pt; mso-fareast-font-family: 'Times New Roman'; mso-ansi-language: EN-US; mso-fareast-language: ZH-CN;" lang="EN-US"><span style="mso-list: Ignore;">5.<span style="font: 7.0pt 'Times New Roman';">   </span></span></span><!--[endif]--><span style="font-size: 10.0pt; mso-fareast-font-family: Calibri; color: #232021; mso-ansi-language: EN-IN; mso-fareast-language: EN-US; mso-bidi-font-weight: bold;">Kumar, S.; Shukla, J.; Kumar, Y.; <span style="mso-spacerun: yes;"> </span>Mandal, K.; Prakash, R.; Ram, P.; Mukhopadhyay, P<em style="mso-bidi-font-style: normal;">.</em> <em>Chem. Sci</em>. </span><strong style="mso-bidi-font-weight: normal;"><span style="font-size: 10.0pt; mso-fareast-font-family: Calibri; color: #232021; mso-ansi-language: EN-IN; mso-fareast-language: EN-US;">2019</span></strong><span style="font-size: 10.0pt; mso-fareast-font-family: Calibri; color: #232021; mso-ansi-language: EN-IN; mso-fareast-language: EN-US; mso-bidi-font-weight: bold;">, <em>10</em>, 6482.</span></p>